GUYA posted some great articles on the topic. I read through some of them, and it is clear that estate planning can be really complex if you live abroad. Many factors (heirs, citizenship of heirs, amount of assets, domicile status, . . . ) all impact the best solution to estate planning.
A US trust for a US citizen living in the UK can be problematic. Whether it is or not is dependent on many factors - wording of trust, if you are UK domiciled or not, if the trust was created before you lived in the UK or not, how long you have lived in the UK, and the list goes on. That's why it's important, in my opinion, to seek legal and tax counsel on how best to plan YOUR estate.
In your situation, you should at least document your US assets so your family knows what you own. Make sure your beneficiaries are listed on all accounts. Children can be listed as secondary if you have someone else listed as primary such as a spouse. If you have a financial advisor, consider giving him or her that information too. My family knows that if anything happened to me and my spouse, they should contact my financial advisor who has a copy of my living trust and list of assets.
Given how young your children are, it is also important to document who you would like custody to go to and if possible ensure your family will have the financial resources they need - consider life insurance.